I have NES, SNES GBA and Megadrive emulators running on it. They're all very good and accessible from home screen once you install banners for them.
ScummVM is particularly great on Wii. Point'n'click with Wiimote is not just novel, it's actually a good match for the controller. Everything up to Monkey Island 3 runs very well with it.
I wouldn't bother actually emulating any computers, there are better solutions for that.
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